Development and application of advanced oxidation technology based on sulfate radical
WANG Xing-liang1, LI Xiao-liang1, WANG Zi2, ZHENG Xing1, LU Si-jia1, ZHU Hui-liang2, SHAO Fei2
1. State Key Laboratory of Eco-hydraulics in Northwest Arid Region of China, Xi'an University of Technology, Xi'an 710048, China; 2. China National Center for Quality Supervision and Inspection of Environmental Protection Equipment, Yixing 214200, China
Abstract: Advanced oxidation technologies based on sulfate radical have developed rapidly in recent years.Various activation methods for persulfate are reviewed systemically,and their advantages and disadvantages are compared and analyzed.Meanwhile,the application of sulfate radical based advanced oxidation technology in the field of environment governance is described.The application prospect and development trend of the technology are also expected.
王行梁, 李晓良, 王子, 郑兴, 路思佳, 朱惠良, 邵飞. 硫酸根自由基高级氧化技术的发展及应用[J]. 现代化工, 2020, 40(S1): 49-53.
WANG Xing-liang, LI Xiao-liang, WANG Zi, ZHENG Xing, LU Si-jia, ZHU Hui-liang, SHAO Fei. Development and application of advanced oxidation technology based on sulfate radical. Modern Chemical Industry, 2020, 40(S1): 49-53.
Guo C,Wang K,Hou S,et al.H2O2 and/or TiO2 photocatalysis under UV irradiation for the removal of antibiotic resistant bacteria and their antibiotic resistance genes[J].Journal of Hazardous Materials,2017,323(Part B):710-718.
Fang Z,Chelme-Ayala P,Shi Q,et al.Degradation of naphthenic acid model compounds in aqueous solution by UV activated persulfate:Influencing factors,kinetics and reaction mechanisms[J].Chemosphere,2018,211:271-277.
[5]
Hori H,Yamamoto A,Hayakawa E,et al.Efficient decomposition of environmentally persistent perfluorocarboxylic acids by use of persulfate as a photochemical oxidant[J].Environmental Science & Technology,2005,39(7):2383-2388.
Wang Y,Chu W.Degradation of 2,4,5-trichlorophenoxyacetic acid by a novel electro-Fe(Ⅱ)/oxone process using iron sheet as the sacrificial anode[J].Water Research,2011,45(13):3883-3889.
[8]
Farhat A,Keller J,Tait S,et al.Removal of persistent organic contaminants by electrochemically activated sulfate[J].Environmental Science & Technology,2015,49(24):14326-14333.
[9]
邹徐.BDD电极电化学氧化去除水中典型农药特性及机理研究[D].长沙:湖南大学,2018.
[10]
Aseev G,Batoeva A,Sizykh R,et al.Sono-photocatalytic degradation of 4-chlorophenolinaqueous solutions[J].Russian Journal of Physical Chemistry A,2018,92(6):1813-1819.
[11]
王倩.水力空化强化过硫酸盐氧化处理染料废水的效能和机理研究[D].杭州:浙江工商大学,2019.
[12]
Angkaew A,Sakulthaew C,Satapanajaru T,et al.UV-activated persulfate oxidation of 17β-estradiol:Implications for discharge water remediation[J].Journal of Environmental Chemical Engineering,2019,7(2):2213-2221.
[13]
Furman O,Teela A,Watts A.Mechanism of base activation of persulfate[J].Environmental Science & Technology,2010,44(16):6423-6428.
Peng W,Liu J,Li C,et al.A multipath peroxymonosulfate activation process over supported by magnetic CuO-Fe3O4 nanoparticles for efficient degradation of 4-chlorophenol[J].Korean Journal of Chemical Engineering,2018,35(8):1662-1672.
[16]
Liang C,Lin Y T,Shin W H.Persulfate regeneration of trichloroethylene spent activated carbon[J].Journal of Hazardous Materials,2009,168(1):187-192.
[17]
Yin R,Guo W,Wang H,et al.Singlet oxygen-dominated peroxydisulfate activation by sludge derived biochar for sulfamethoxazole degradation through a nonradical oxidation pathway:Performance and mechanism[J].Chemical Engineering Journal,2019,357:589-599.
[18]
Lin K Y A,Chen S Y,Jochems A P.Zirconium-based metal organic frameworks:Highly selective adsorbents for removal of phosphate from water and urine[J].Materials Chemistry and Physics,2015,160:168-176.
[19]
Pu M,Guan Z,Ma Y,et al.Synthesis of iron-based metal-organic framework MIL-53 as an efficient catalyst to activate persulfate for the degradation of Orange G in aqueous solution[J].Applied Catalysis A,General,2018,549:82-92.
[20]
Li H,Tian J,Zhu Z,et al.Magnetic nitrogen-doped nanocarbons for enhanced metal free catalytic oxidation:Integrated experimental and theoretical investigations for mechanism and application[J].Chemical Engineering Journal,2018,354:507-516.
Chu L,Zhuan R,Chen D,et al.Degradation of macrolide antibiotic erythromycin and reduction of antimicrobial activity using persulfate activated by gamma radiation in different water matrices[J].Chemical Engineering Journal,2019,361:156-166.
[23]
Takdastan A,Kakavandi B,Azizi M.Efficient activation of peroxymonosulfate by using ferroferric oxide supported on carbon UV/US system:A new approach into catalytic degradation of bispheno-l A[J].Chemical Engineering Journal,2018,331:729-743.