DBD等离子体协同催化降解甲醛气体及光谱诊断研究

邢倩云, 李茹, 杨鑫, 梁煜, 冯燕

现代化工 ›› 2022, Vol. 42 ›› Issue (10) : 120 -125.

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现代化工 ›› 2022, Vol. 42 ›› Issue (10) : 120-125. DOI: 10.16606/j.cnki.issn0253-4320.2022.10.023
科研与开发

DBD等离子体协同催化降解甲醛气体及光谱诊断研究

    邢倩云, 李茹, 杨鑫, 梁煜, 冯燕
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DBD plasma co-catalytic degradation of formaldehyde gas and spectral diagnosis

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摘要

采用介质阻挡放电(DBD)等离子体协同催化降解甲醛气体,考察了放电功率、初始质量浓度、气体流量对甲醛的降解效率、能量效率和生成的臭氧(O3)质量浓度的影响。结果表明,在初始质量浓度为41.12 mg/m3、气体体积流量为 0.7 L/min、放电功率为30 W的最佳反应条件下加入Mn-TiO2/γ-Al2O3催化剂后,甲醛的降解效率和反应器的能量效率分别高达90.71%和0.052 g/(kW·h),O3质量浓度下降至121.957 mg/m3

Abstract

Dielectric barrier discharge (DBD) plasma is used to co-catalyze the degradation of formaldehyde gas,and the effects of reaction conditions on the degradation efficiency of formaldehyde,the energy efficiency of reactor and the mass concentration of ozone formed are analyzed.The optimal reaction conditions are determined as follows:the initial concentration is 41.12 mg·m-3,the gas volume flow is 0.7 L·min-1,and the discharge power is 30 W.Under these conditions and over Mn-TiO2/γ-Al2O3 catalyst,the degradation efficiency of formaldehyde reaches as high as 90.71%,the energy efficiency of the reactor reaches 0.052 g·(kW·h)-1,while the mass concentration of O3 generated drops to 121.957 mg·m-3.

关键词

介质阻挡放电(DBD) / 等离子体诊断 / 催化剂 / 甲醛气体

Key words

dielectric barrier discharge (DBD) / plasma diagnosis / catalyst / formaldehyde gas

Author summay

邢倩云(1995-),女,硕士研究生,主要研究方向为低温等离子体降解VOCs,1285735217@qq.com

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DBD等离子体协同催化降解甲醛气体及光谱诊断研究[J]. 现代化工, 2022, 42(10): 120-125 DOI:10.16606/j.cnki.issn0253-4320.2022.10.023

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