利用过量浸渍法制备了Fe-ZSM-5催化剂，考察制备条件和反应条件对Fe-ZSM-5催化剂在甲基橙溶液中降解过程的影响，同时用XRD和XPS对催化剂的表面性质进行表征。结果表明，Fe₂O₃是催化剂的主要活性位，能够显著提高甲基橙催化降解的效果；制备条件和反应条件对Fe-ZSM-5催化降解反应均具有较大的影响。最佳制备条件为：煅烧温度为400℃，Fe负载量为1%；最佳反应工艺条件为：催化剂质量为1.5 g，Fe与H₂O₂摩尔比为1：6，pH为3。

Fe-ZSM-5 catalyst is prepared by means of overdose dip-molding method.The degradation process of methyl orange solution is used to evaluate the effects of preparation conditions for Fe-ZSM-5 catalyst and reaction conditions.Characterization on surface property of the catalyst is conducted by means of XRD and XPS.Experimental results show that Fe₂O₃ is the major active sites of the catalyst and can promote remarkably the degradation efficiency of methyl orange.The preparation conditions for Fe-ZSM-5 catalyst and reaction conditions both have significant influences on the degradation reaction.The optimal preparation conditions include a calcination temperature of 400℃ and 1% Fe loading amount,while the optimal reaction conditions are as follows:the adding amount of catalyst is 1.5 g,the molar ratio of Fe to H₂O₂ is 1:6 and pH is 3.

陈嘉瑾(1997-),男,本科在读,研究方向为水处理技术,540126337@qq.com