PDF (1757K)
摘要
负载型金(Au)纳米催化剂对CO氧化反应过程具有较高的催化活性,而其负载载体的物化性质对Au催化活性的提升有显著影响。系统地总结了几种常见的Au催化剂载体(活性载体:TiO2、CeO2以及Co3O4;惰性载体:SiO2和Al2O3)在协调Au催化氧化CO过程中的催化性能及相关的作用机制,重点分析了各载体对催化性能的影响,对负载型Au催化剂载体的选择及设计提供指导,并对未来Au催化剂的发展方向做了展望。
Abstract
Supported gold (Au) nano-catalyst has high catalytic activity for CO oxidation reaction process,and the physical and chemical properties of the carrier used to support Au have a significant impact on the improvement of Au's catalytic activity.Several common carriers for supporting Au catalyst,including active carriers such as TiO2,CeO2 and Co3O4;inert carriers such as SiO2 and Al2O3,are systematically summarized in terms of their catalytic performance and related mechanism in coordinating Au to catalyze the oxidation of CO.The influences of each carrier on the catalytic performance of the catalyst are emphatically analyzed,and the development direction of Au catalysts in the future is prospected.It provides guidance for the selection and design of carrier in supported Au catalyst,and gives prospects on the development directions of Au-based catalyst in the future.
关键词
CO氧化
/
催化性能
/
反应机理
/
载体
/
Au催化剂
Key words
CO oxidation
/
catalytic performance
/
reaction mechanism
/
support
/
Au-based catalyst
Author summay
吴辰(2000-),女,硕士生,研究方向为生物质科学与工程。
用于CO氧化的Au催化剂载体研究进展[J].
, 2023, 43(S1): 11-16,23 DOI:10.16606/j.cnki.issn0253-4320.2023.S1.003