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摘要
重点介绍了近10年来用于介质阻挡放电(DBD)辅助催化CO2甲烷化的镍基催化剂的研究成果,包括不同等离子体工艺参数下的催化剂活性,同时涉及催化剂的活化方式、载体、助剂等实验条件对催化效果的影响,揭示了介质阻挡放电辅助催化CO2甲烷化中等离子体与催化剂的协同效应和反应机理。最后针对DBD等离子体辅助催化体系目前所面临的挑战,提出了新的展望。
Abstract
This review focuses on the research progress in the nickel-based catalysts for dielectric barrier discharge (DBD) assisted catalysis of CO2 methanation in the past ten years,including the catalyst activity under different plasma process parameters,and the influences of catalyst activation mode,support,additives,and other experimental conditions on the catalytic effect.The synergistic effect and reaction mechanism of plasma and catalyst in CO2 methanation assisted by DBD are revealed.Finally,a new prospect is proposed for the challenges of the DBD plasma-assisted catalysis system.
关键词
非热等离子体
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协同效应
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CO2甲烷化
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镍基催化剂
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介质阻挡放电
Key words
non thermal plasma
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synergistic effect
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CO2 methanation
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nickel-based catalysts
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dielectric barrier discharge
Author summay
介质阻挡放电辅助催化CO2甲烷化的研究[J].
, 2023, 43(10): 52-57 DOI:10.16606/j.cnki.issn0253-4320.2023.10.010