Please wait a minute...
 
最新公告: 重要提醒:骗子冒充编辑部要求加作者微信,谨防上当!   关于暑假、寒假期间版面费发票及期刊样刊延迟邮寄的通知    
现代化工  2018, Vol. 38 Issue (4): 18-21    DOI: 10.16606/j.cnki.issn0253-4320.2018.04.005
  技术进展 本期目录 | 过刊浏览 | 高级检索 |
酸/碱/盐改性石墨相氮化碳光催化材料研究进展
张西标, 宋海岩, 孙才英, 韩福芹, 李博伦
东北林业大学理学院, 黑龙江 哈尔滨 150040
Research progress in acid/alkali/salt modified graphitic carbon nitride photocatalytic materials
ZHANG Xi-biao, SONG Hai-yan, SUN Cai-ying, HAN Fu-qin, LI Bo-lun
College of Science, Northeast Forestry University, Harbin 150040, China
下载:  PDF (1280KB) 
输出:  BibTeX | EndNote (RIS)      
摘要 介绍了近年来国内外利用酸、碱、盐修饰或改性g-C3N4的掺杂物种、工艺路线及其对理化性质的改善,同时对其在光催化领域中的应用与光催化性能上的提升进行了总结。
服务
把本文推荐给朋友
加入引用管理器
E-mail Alert
RSS
作者相关文章
张西标
宋海岩
孙才英
韩福芹
李博伦
关键词:  石墨相氮化碳        改性    
Abstract: This paper reviews comprehensively the doping species and preparation techniques in using acid/alkali/salt to modify graphitic carbon (g-C3N4),as well as the resulted physicochemical properties improvement at home and abroad in recent years.Meanwhile,the applications of the modified g-C3N4 in the photocatalysis aspect and the enhanced photocatalytic activity of this material family are summarized.
Key words:  graphitic carbon nitride    acid    alkali    salt    modification
收稿日期:  2017-09-28                出版日期:  2018-04-20
TM23  
基金资助: 中央高校基本科研业务费专项资金资助(2572017CB31);中国博士后科学基金第60批面上资助项目(2016M601403)
通讯作者:  宋海岩(1981-),男,博士,讲师,主要从事多孔材料合成与应用方面的研究,通讯联系人,0451-82190679,chem-shy@163.com;孙才英(1964-),女,博士,教授,从事含磷阻燃剂方向的研究,通讯联系人,0451-82190679,sundeyee@126.com。    E-mail:  chem-shy@163.com;sundeyee@126.com
作者简介:  张西标(1991-),男,硕士生
引用本文:    
张西标, 宋海岩, 孙才英, 韩福芹, 李博伦. 酸/碱/盐改性石墨相氮化碳光催化材料研究进展[J]. 现代化工, 2018, 38(4): 18-21.
ZHANG Xi-biao, SONG Hai-yan, SUN Cai-ying, HAN Fu-qin, LI Bo-lun. Research progress in acid/alkali/salt modified graphitic carbon nitride photocatalytic materials. Modern Chemical Industry, 2018, 38(4): 18-21.
链接本文:  
http://www.xdhg.com.cn/CN/10.16606/j.cnki.issn0253-4320.2018.04.005  或          http://www.xdhg.com.cn/CN/Y2018/V38/I4/18
[1] Zhao Z,Sun Y,Dong F.Graphitic carbon nitride based nanocomposites:A review[J].Nanoscale,2015,7(1):15-37.
[2] Cheng N,Tian J,Liu Q,et al.Au-nanoparticle-loaded graphitic carbon nitride nanosheets:Green photocatalytic synthesis and application toward the degradation of organic pollutants[J].ACS Appl Mater Interfaces,2013,5(15):6815-6819.
[3] Chen P,Li K,Yu Y,et al.Cobalt-doped graphitic carbon nitride photocatalysts with high activity for hydrogen evolution[J].Applied Surface Science,2017,392:608-615.
[4] He Q,Zhou F,Zhan S,et al.Enhancement of photocatalytic and photoelectrocatalytic activity of Ag modified Mpg-C3N4 composites[J].Applied Surface Science,2017,391:423-431.
[5] Yan H,Yang H.TiO2-g-C3N4 composite materials for photocatalytic H2 evolution under visible light irradiation[J].Journal of Alloys and Compounds,2011,509(4):26-29.
[6] Ge L,Han C,Xiao X,et al.Synthesis and characterization of composite visible light active photocatalysts MoS2-g-C3N4 with enhanced hydrogen evolution activity[J].International Journal of Hydrogen Energy,2013,38(17):6960-6969.
[7] Han C,Ge L,Chen C,et al.Novel visible light induced Co3O4-g-C3N4 heterojunction photocatalysts for efficient degradation of methyl orange[J].Applied Catalysis B:Environmental,2014,147:546-553.
[8] Liu G,Niu P,Sun C,et al.Unique electronic structure induced high photoreactivity of sulfur-doped graphitic C3N4[J].ACS Publications,2010,132(33):11642-11648.
[9] Qiu P,Xu C,Chen H,et al.One step synthesis of oxygen doped porous graphitic carbon nitride with remarkable improvement of photo-oxidation activity:Role of oxygen on visible light photocatalytic activity[J].Applied Catalysis B:Environmental,2017,206:319-327.
[10] Kwon K,Sa Y J,Cheon J Y,et al.Ordered mesoporous carbon nitrides with graphitic frameworks as metal-free,highly durable,methanol-tolerant oxygen reduction catalysts in an acidic medium[J].Langmuir,2012,28(1):991-996.
[11] Peer M,Lusardi M,Jensen K F.Facile soft-templated synthesis of high-surface area and highly porous carbon nitrides[J].Chemistry of Materials,2017,29(4):1496-1506.
[12] Goettmann F,Fischer A,Antonietti M,et al.Chemical synthesis of mesoporous carbon nitrides using hard templates and their use as a metal-free catalyst for friedel-crafts reaction of benzene[J].Angew Chem Int Ed Engl,2006,45(27):4467-4471.
[13] Yang S,Gong Y,Zhang J,et al.Exfoliated graphitic carbon nitride nanosheets as efficient catalysts for hydrogen evolution under visible light[J].Adv Mater,2013,25(17):2452-2456.
[14] Tian J,Liu Q,Ge C,et al.Ultrathin graphitic carbon nitride nanosheets:A low-cost,green,and highly efficient electrocatalyst toward the reduction of hydrogen peroxide and its glucose biosensing application[J].Nanoscale,2013,5(19):8921-8924.
[15] Tian J,Liu Q,Asiri A M,et al.Ultrathin graphitic carbon nitride nanosheets:A novel peroxidase mimetic,Fe doping-mediated catalytic performance enhancement and application to rapid,highly sensitive optical detection of glucose[J].Nanoscale,2013,5(23):11604-11609.
[16] Xu C,Li K,Zhang W.Enhancing visible light photocatalytic activity of nitrogen-deficient g-C3N4 via thermal polymerization of acetic acid-treated melamine[J].Journal of Colloid and Interface Science,2017,495:27-36.
[17] Wu M,Yan J M,Zhang X W,et al.Synthesis of g-C3N4 with heating acetic acid treated melamine and its photocatalytic activity for hydrogen evolution[J].Applied Surface Science,2015,354:196-200.
[18] Han X,Tian L,Jiang H,et al.Facile transformation of low cost melamine-oxalic acid into porous graphitic carbon nitride nanosheets with high visible-light photocatalytic performance[J].Royal Society of Chemistry,2017,7(24):14372-14381.
[19] Zhou Y,Zhang L,Huang W,et al.N-doped graphitic carbon-incorporated g-C3N4 for remarkably enhanced photocatalytic H2 evolution under visible light[J].Carbon,2016,99:111-117.
[20] 吴思展.类石墨氮化碳(g-C3N4)的合成、加工处理、修饰及其光催化性能的研究[D].广州:华南理工大学,2014.
[21] Xu J,Zhang L,Shi R,et al.Chemical exfoliation of graphitic carbon nitride for efficient heterogeneous photocatalysis[J].Journal of Materials Chemistry A,2013,1(46):14766-14772.
[22] Shi L,Wang F,Liang L,et al.In site acid template induced facile synthesis of porous graphitic carbon nitride with enhanced visible-light photocatalytic activity[J].Catalysis Communications,2017,89:129-132.
[23] Raevskaya A E,Panasiuk Y V,Korzhak G V,et al.Photocatalytic H2 production from aqueous solutions of hydrazine and its derivatives in the presence of nitric-acid-activated graphitic carbon nitride[J].Catalysis Today,2017,284:229-235.
[24] Zhu Y,Zhu M,Kang L,et al.Phosphotungstic acid supported on mesoporous graphitic carbon nitride as catalyst for oxidative desulfurization of fuel[J].Industrial & Engineering Chemistry Research,2015,54(7):2040-2047.
[25] Xu J,Shang J,Jiang Q,et al.Facile alkali-assisted synthesis of g-C3N4 materials and their high-performance catalytic application in solvent-free cycloaddition of CO2 to epoxides[J].Royal Society of Chemistry,2016,6(60):55382-55392.
[26] Sun Z,Fischer J M T A,Li Q,et al.Enhanced CO2 photocatalytic reduction on alkali-decorated graphitic carbon nitride[J].Applied Catalysis B:Environmental,2017,216:146-155.
[27] Cheng F,Yan J,Zhou C,et al.An alkali treating strategy for the colloidization of graphitic carbon nitride and its excellent photocatalytic performance[J].Journal of Colloid and Interface Science,2016,468:103-109.
[28] Zhang J,Hu S,Wang Y.A convenient method to prepare a novel alkali metal sodium doped carbon nitride photocatalyst with a tunable band structure[J].Royal Society of Chemistry,2014,4(108):62912-62919.
[29] Hu S,Li F,Fan Z,et al.Band gap-tunable potassium doped graphitic carbon nitride with enhanced mineralization ability[J].Dalton Trans,2015,44(3):1084-1092.
[30] Chen D,Yang J,Ding H.Synthesis of nanoporous carbon nitride using calcium carbonate as templates with enhanced visible-light photocatalytic activity[J].Applied Surface Science,2017,391:384-391.
[31] Gibot P,Schnell F,Spitzer D.Enhancement of the graphitic carbon nitride surface properties from calcium salts as templates[J].Microporous and Mesoporous Materials,2016,219:42-47.
[32] Yuan B,Zou X,Yan T,et al.Green synthesis of graphitic carbon nitride nanodots using sodium chloride template[J].Journal of Nanoparticle Research,2016,18(5):109-117.
[33] Shang Y,Ma Y,Chen X,et al.Effect of sodium doping on the structure and enhanced photocatalytic hydrogen evolution performance of graphitic carbon nitride[J].Molecular Catalysis,2017,433:128-135.
[34] Wu M,Yan J M,Tang X N,et al.Synthesis of potassium-modified graphitic carbon nitride with high photocatalytic activity for hydrogen evolution[J].Chem Sus Chem,2014,7(9):2654-2658.
[35] 李欣蔚,张会均,文莉,等.K掺杂C3N4的原位合成、禁带结构解析及其可见光催化性能增强机制[J].中国科学通报,2016,61(24):2707-2716.
[1] 王峰. MTP工艺副产轻质油在HZSM-5上催化裂解行为的研究[J]. 现代化工, 2018, 38(9): 122-126.
[2] 陶梅, 罗桂玲, 罗霄, 任晗, 罗跃. 钻井液用聚合物弱凝胶的研制与性能研究[J]. 现代化工, 2018, 38(9): 132-135,137.
[3] 颜鑫, 卢云峰. 碳化气浓度渐降模式对纳米碳酸钙碳化过程的影响研究[J]. 现代化工, 2018, 38(9): 180-183.
[4] 刘艳杰, 王犇, 潘高峰. 乙酸异丙酯回收工艺模拟与优化[J]. 现代化工, 2018, 38(9): 215-218.
[5] 李强, 钱俊峰, 查杰, 左士祥, 姚超. 一步水热法制备ATP/CuFe2O4纳米复合材料及其催化还原对硝基苯酚[J]. 现代化工, 2018, 38(9): 168-173.
[6] 刘婷婷, 乔建江. 复合氢氧化铝-季戊四醇的制备及其应用研究[J]. 现代化工, 2018, 38(9): 155-159.
[7] 姜巧娟, 李华, 刘彦平, 郑先君, 付长亮, 刘从军. Pt/TiO2的制备及其在利用废水中有机酸产氢中的性能研究[J]. 现代化工, 2018, 38(9): 160-163.
[8] 杨凤丽, 仝雪, 秦丽珍, 郑纯智, 夏斐斐. 铌类固体酸催化糖转化5-羟甲基糠醛研究进展[J]. 现代化工, 2018, 38(9): 28-32.
[9] 王海坤, 邱祖民, 熊凌亨, 王一斐, 宁峰. 硅藻土/羧甲基纤维素钠有机-无机高吸水树脂的制备[J]. 现代化工, 2018, 38(9): 68-71,73.
[10] 韩英, 郝文婷, 魏旭青, 王明, 孙彤, 谢晶, 励建荣. CaCO3添加量对原位改性纳米CaCO3/壳聚糖复合涂膜理化性能的影响[J]. 现代化工, 2018, 38(9): 77-80.
[11] 刘梦真, 常艳, 张文, 王宇新. 印刷电路板酸性氯化铜蚀刻液电解再生的优化流程[J]. 现代化工, 2018, 38(9): 204-208.
[12] 刘雅, 石鹏, 王静康, 龚俊波. 长链二元酸的制备与精制研究进展[J]. 现代化工, 2018, 38(8): 43-47.
[13] 王嘉欣, 唐善法, 赵成洋, 蒲明政, 樊英凯, 郑雅慧. 磺酸盐Gemini表面活性剂的合成及性能研究[J]. 现代化工, 2018, 38(8): 117-120.
[14] 陈柳, 魏永梅, 王涛, 田恒水. 异山梨醇型聚碳酸酯的共聚改性研究[J]. 现代化工, 2018, 38(8): 130-134.
[15] 尹俊华, 薄翠梅, 黄燕, 丁帅. 醋酸甲酯水解过程厂级经济控制[J]. 现代化工, 2018, 38(8): 221-226.
[1] . [J]. Modern Chemical Industry, 2015, 35(11): 77 -80 .
[2] . [J]. Modern Chemical Industry, 2015, 35(12): 128 -130,132 .
[3] . [J]. Modern Chemical Industry, 2017, 37(6): 103 -0106,108 .
[4] . [J]. , 2003, 23(5): 0 .
[5] . [J]. , 2009, 29(6): 0 .
[6] . [J]. , 2010, 30(3): 0 .
[7] . [J]. , 2010, 30(7): 0 .
[8] . [J]. , 2007, 27(2): 0 .
[9] . [J]. Modern Chemical Industry, 2014, 34(2): 131 -133 .
[10] . [J]. Modern Chemical Industry, 2014, 34(4): 14 -16 .
Viewed
Full text


Abstract

Cited

  Shared   
  Discussed   
京ICP备09035943号-37
版权所有 © 《现代化工》编辑部
本系统由北京玛格泰克科技发展有限公司设计开发 技术支持:support@magtech.com.cn