Please wait a minute...
 
最新公告: 重要提醒:骗子冒充编辑部要求加作者微信,谨防上当!   关于暑假、寒假期间版面费发票及期刊样刊延迟邮寄的通知    
现代化工  2019, Vol. 39 Issue (7): 75-78    DOI: 10.16606/j.cnki.issn0253-4320.2019.07.016
  技术进展 本期目录 | 过刊浏览 | 高级检索 |
氧化法在汽油深度脱硫中的研究进展
梅学赓, 吴明清, 李涛
中国石油化工股份有限公司石油化工科学研究院, 北京 100083
Research progress in oxidation method for deep desulfurization of gasoline
MEI Xue-geng, WU Ming-qing, LI Tao
SINOPEC Research Institute of Petroleum Processing, Beijing 100083, China
下载:  PDF (1282KB) 
输出:  BibTeX | EndNote (RIS)      
摘要 综述了分子氧氧化、H2O2氧化以及其他催化氧化法在汽油脱硫领域的研究进展,并对氧化法脱硫技术未来发展做出展望。
服务
把本文推荐给朋友
加入引用管理器
E-mail Alert
RSS
作者相关文章
梅学赓
吴明清
李涛
关键词:  汽油  氧气  双氧水  氧化脱硫    
Abstract: This paper summarizes the research progress in removing sulfur-containing compounds from gasoline via oxidative desulfurization methods,including hydrogen peroxide oxidation,oxygen molecular oxidation and other oxidation methods.And the developing prospect of oxidant desulfurization technology in the future is also presented.
Key words:  gasoline    oxygen    hydrogen peroxide    oxidation desulfurization
收稿日期:  2018-12-20      修回日期:  2019-05-05           出版日期:  2019-07-20
TE-624  
通讯作者:  吴明清(1963-),男,博士,教授级高工,研究方向为轻质油品脱硫,通讯联系人,wumq.ripp@sinopec.com。    E-mail:  wumq.ripp@sinopec.com
作者简介:  梅学赓(1993-),男,硕士生
引用本文:    
梅学赓, 吴明清, 李涛. 氧化法在汽油深度脱硫中的研究进展[J]. 现代化工, 2019, 39(7): 75-78.
MEI Xue-geng, WU Ming-qing, LI Tao. Research progress in oxidation method for deep desulfurization of gasoline. Modern Chemical Industry, 2019, 39(7): 75-78.
链接本文:  
http://www.xdhg.com.cn/CN/10.16606/j.cnki.issn0253-4320.2019.07.016  或          http://www.xdhg.com.cn/CN/Y2019/V39/I7/75
[1] Campos-Martin J M,Capel-Sanchez M C,Fierro J L G.Highly efficient deep desulfurization of fuels by chemical oxidation[J].Green Chemistry,2004,6(11):557-562.
[2] 仇玄.2016年我国成品油市场回顾及2017年展望[J].中国石油和化工经济分析,2017,(1):23-26.
[3] Khayyat S,Selva Roselin L.Photocatalytic degradation of benzothiophene and dibenzothiophene using supported gold nanoparticle[J].Journal of Saudi Chemical Society,2017,21(3):349-357.
[4] 秦如意,张晓静,刘金龙.FCC汽油吸附脱硫工艺的研究[J].石油炼制与化工,2003,34(3):24-28.
[5] Debabov V G.Microbial desulfurization of motor fuel[J].Applied Biochemistry & Microbiology,2010,46(8):733-738.
[6] Zhang S,Zhang Q L,Zhang A.Extractive desulfurization and denitrogenation of fuels using ionic liquids[J].Ind Eng Chem,2004,43(2):614-622.
[7] Me H,Mei B,Yen W.A new method for obtaining ultra-low sulfur diesel fuel via ultrasound assisted oxidative desulfurization[J].Fuel,2003,82(4):405-414.
[8] Hirai T,Ken Ogawa,Komasawa A.Desulfurization process for dibenzothiophenes from light oil by photochemical reaction and liquid-liquid extraction[J].Industrial & Engineering Chemistry Research,1996,35(2):586-589.
[9] Murata S,Murata K,Kidena K E A.A novel oxidative desulfurization system for diesel fuels with molecular oxygen in the presence of cobalt catalysts and aldehydes[J].Energy & Fuels,2004,18(1):116-121.
[10] Sampanthar J T,Xiao H,Dou J.A novel oxidative desulfurization process to remove refractory sulfur compounds from diesel fuel[J].Applied Catalysis B Environmental,2006,63(1):85-93.
[11] 熊杰明,迟姚玲,胡应喜,等.过氧化氢/甲酸/硫酸体系氧化脱硫研究[J].石油化工高等学校学报,2009,22(3):1-4.
[12] Otsuki S,Nonaka T,Takashima N.Oxidative desulfurization of light gas oil and vacuum gas oil by oxidation and solvent extraction[J].Energy & Fuels,2000,14(6):750-753.
[13] Bhasarkar J B,Chakma S,Moholkar V S.Investigations in physical mechanism of the oxidative desulfurization process assisted simultaneously by phase transfer agent and ultrasound[J].Ultrasonics Sonochemistry,2015,24:98-106.
[14] Alvarez-Amparán M A,Cedeño-Caero L,Cortes-Jácome M A,et al.Relationship between the catalytic activity and Mo-V surface species in bimetallic catalysts for the oxidative desulfurization of dibenzothiophenic compounds[J].Reaction Kinetics,Mechanisms and Catalysis,2017,122(2):869-885.
[15] Rabion A,François Fajula,Bernard J R,et al.Method for desulphurizing thiopene derivatives contained in fuels:US,7179368[P].2003-06-05.
[16] Ji H,Sun J,Wu P,et al.Silicotungstic acid immobilized on lamellar hexagonal boron nitride for oxidative desulfurization of fuel components[J].Fuel,2018,213:12-21.
[17] Chen X,Song D,Asumana C,et al.Deep oxidative desulfurization of diesel fuels by Lewis acidic ionic liquids based on 1-n-butyl-3-methylimidazolium metal chloride[J].Journal of Molecular Catalysis A:Chemical,2012,359:8-13.
[18] Ye G,Sun Y,Zhang D,et al.Hierarchical porous titanium terephthalate based material with highly active sites for deep oxidative desulfurization[J].Microporous & Mesoporous Materials,2018,270:241-247.
[19] Wang D,Qian E W,Amano H,et al.Oxidative desulfurization of fuel oil[J].Applied Catalysis A:General,2003,253(1):91-99.
[1] 叶芳芳, 张帅, 李长刚, 聂丽君. 生产清洁汽油技术的研究进展[J]. 现代化工, 2019, 39(7): 71-74,76.
[2] 程光南, 张孔远, 魏麟骄. FCC汽油馏分在Ni/Al2O3催化剂上加氢脱硫醇的研究[J]. 现代化工, 2019, 39(2): 159-161,163.
[3] 刘剑, 陈丽晶, 汲永钢, 万书宝, 孙淑坤, 代跃利. 乙烯焦油加氢制汽油试验研究[J]. 现代化工, 2019, 39(2): 189-191.
[4] 杨乾坚, 张俊杰, 潘登, 杨旭东. 催化轻汽油溶剂抽提脱硫工艺与醚化LNE-2工艺在轻汽油醚化装置上的联合应用[J]. 现代化工, 2019, 39(1): 205-208.
[5] 宋利军. 甲醇作为车用汽油调合组分的利弊分析[J]. 现代化工, 2018, 38(8): 12-16.
[6] 张言斌, 李芹, 钟黄亮, 罗聃, 周红军, 周广林. Fe3O4@SiO2-Cu复合磁性纳米粒子的制备及其脱硫性能的研究[J]. 现代化工, 2018, 38(6): 101-105.
[7] 田欢, 杜岳, 郭振冉, 杜小弟. 分级多孔HPW/TiO2催化剂的合成及其氧化脱硫性能[J]. 现代化工, 2018, 38(6): 148-153.
[8] 宁海涛. 原料预热温度降低对催化裂化装置的影响[J]. 现代化工, 2018, 38(5): 198-200.
[9] 徐竞帆, 李爱蓉, 蒋乐乐. 磷钨酸盐离子液体合成WO3-SiO2及催化模拟油氧化脱硫[J]. 现代化工, 2018, 38(4): 105-109.
[10] 刘思彤, 石薇薇, 曹祖宾, 吴迪, 姜永辉. FCC汽油重馏分氧化-吸附脱硫的研究[J]. 现代化工, 2018, 38(4): 148-151,153.
[11] 张瑞风, 孟凡东, 闫鸿飞, 孙世源, 张亚西. 催化裂化系统压力的影响及选择[J]. 现代化工, 2018, 38(3): 207-209,211.
[12] 吴凤芹, 吕新刚, 左士祥, 李霞章, 姚超. 超细钨酸铋/凹凸棒石光催化剂的制备及其脱硫性能[J]. 现代化工, 2018, 38(11): 72-76.
[13] 门秀杰, 孙海萍, 雷强, 张胜军, 荆延妮. 我国推广乙醇汽油的进展、影响及应对建议[J]. 现代化工, 2018, 38(11): 8-11,13.
[14] 马好文, 宋健强, 胡晓丽, 梁顺琴, 孙利民, 冯辉霞. 环丁砜对裂解汽油一、二段加氢催化剂的影响[J]. 现代化工, 2017, 37(8): 113-116,118.
[15] 闫鸿飞, 孟凡东, 王龙延, 张亚西, 孙世源. 加氢催化柴油进第二提升管多产汽油工艺开发与应用[J]. 现代化工, 2017, 37(7): 175-178.
[1] . [J]. Modern Chemical Industry, 2015, 35(11): 77 -80 .
[2] . [J]. Modern Chemical Industry, 2017, 37(5): 71 -75 .
[3] . [J]. , 2002, 22(4): 0 .
[4] . [J]. , 2003, 23(5): 0 .
[5] . [J]. , 2011, 31(4): 0 .
[6] . [J]. , 2011, 31(6): 0 .
[7] . [J]. , 2009, 29(3): 0 .
[8] . [J]. , 2009, 29(12): 0 .
[9] . [J]. Modern Chemical Industry, 2014, 34(2): 1 -8 .
[10] . [J]. Modern Chemical Industry, 2014, 34(4): 14 -16 .
Viewed
Full text


Abstract

Cited

  Shared   
  Discussed   
京ICP备09035943号-37
版权所有 © 《现代化工》编辑部
本系统由北京玛格泰克科技发展有限公司设计开发 技术支持:support@magtech.com.cn